A Valuable Biochar from Poplar Catkins with High Adsorption Capacity for Both Organic Pollutants and Inorganic Heavy Metal Ions.
Identifieur interne : 001554 ( Main/Exploration ); précédent : 001553; suivant : 001555A Valuable Biochar from Poplar Catkins with High Adsorption Capacity for Both Organic Pollutants and Inorganic Heavy Metal Ions.
Auteurs : Xia Liu [République populaire de Chine] ; Ju Sun [République populaire de Chine] ; Shengxia Duan [République populaire de Chine] ; Yanan Wang [République populaire de Chine] ; Tasawar Hayat [Arabie saoudite] ; Ahmed Alsaedi [Arabie saoudite, Pakistan] ; Chengming Wang [République populaire de Chine] ; Jiaxing Li [République populaire de Chine, Arabie saoudite]Source :
- Scientific reports [ 2045-2322 ] ; 2017.
Abstract
In this paper, biochar derived from poplar catkins was used as an economical and renewable adsorbent for adsorption organic and inorganic pollutants such as, dyes, organic compounds, and heavy metal ions from wastewater. Mesoporous activated carbonized poplar catkins (ACPCs) were produced from char as a by-product by carbonized poplar catkins (CPCs). With their high surface area, ACPCs exhibited the maximum adsorption capacities of 71.85 and 110.17 mg/g for the removal of inorganic U(VI) and Co(II). Compared other biochars adsorbents, ACPCs can also adsorb organic pollutants with the maximum adsorption capacities of 534, 154, 350, 148 and 384 mg/g for methylene blue (MB), methyl orange (MO), Congo red (CR), chloramphenicol (CAP) and naphthalene. The adsorption of organic pollutants was fitted with pseudo-first order, pseudo-second order, and intra-particle diffusion kinetic models figure out the kinetic parameters and adsorption mechanisms. Langmuir adsorption isotherm was found to be suitable for Co(II) and U(VI) adsorption and thermodynamic studies indicated adsorption processes to be endothermic and spontaneous. The adsorption process includes both outer-sphere surface complexes and hydrogen-bonding interactions. The results showed that biochar derived from poplar catkins was a potential material to remove pollutants in wastewater.
DOI: 10.1038/s41598-017-09446-0
PubMed: 28855653
PubMed Central: PMC5577165
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China.</nlm:affiliation><country xml:lang="fr" wicri:curation="lc">République populaire de Chine</country><wicri:regionArea>University of Science and Technology of China, Hefei, 230026</wicri:regionArea><wicri:noRegion>230026</wicri:noRegion></affiliation></author><author><name sortKey="Hayat, Tasawar" sort="Hayat, Tasawar" uniqKey="Hayat T" first="Tasawar" last="Hayat">Tasawar Hayat</name><affiliation wicri:level="1"><nlm:affiliation>NAAM Research Group, Faculty of Science, King Abdulaziz University, Jeddah, 21589, Saudi Arabia.</nlm:affiliation><country xml:lang="fr">Arabie saoudite</country><wicri:regionArea>NAAM Research Group, Faculty of Science, King Abdulaziz University, Jeddah, 21589</wicri:regionArea><wicri:noRegion>21589</wicri:noRegion></affiliation></author><author><name sortKey="Alsaedi, Ahmed" sort="Alsaedi, Ahmed" uniqKey="Alsaedi A" first="Ahmed" last="Alsaedi">Ahmed Alsaedi</name><affiliation wicri:level="1"><nlm:affiliation>NAAM Research Group, Faculty of Science, King Abdulaziz University, Jeddah, 21589, Saudi Arabia.</nlm:affiliation><country xml:lang="fr">Arabie saoudite</country><wicri:regionArea>NAAM Research Group, Faculty of Science, King Abdulaziz University, Jeddah, 21589</wicri:regionArea><wicri:noRegion>21589</wicri:noRegion></affiliation><affiliation wicri:level="1"><nlm:affiliation>Department of Mathematics, Quaid-I-Azam University, Islamabad, 44000, Pakistan.</nlm:affiliation><country xml:lang="fr">Pakistan</country><wicri:regionArea>Department of Mathematics, Quaid-I-Azam University, Islamabad, 44000</wicri:regionArea><wicri:noRegion>44000</wicri:noRegion></affiliation></author><author><name sortKey="Wang, Chengming" sort="Wang, Chengming" uniqKey="Wang C" first="Chengming" last="Wang">Chengming Wang</name><affiliation wicri:level="1"><nlm:affiliation>University of Science and Technology of China, Hefei, 230026, P.R. China.</nlm:affiliation><country xml:lang="fr" wicri:curation="lc">République populaire de Chine</country><wicri:regionArea>University of Science and Technology of China, Hefei, 230026</wicri:regionArea><wicri:noRegion>230026</wicri:noRegion></affiliation></author><author><name sortKey="Li, Jiaxing" sort="Li, Jiaxing" uniqKey="Li J" first="Jiaxing" last="Li">Jiaxing Li</name><affiliation wicri:level="1"><nlm:affiliation>Institute of Plasma Physics, Chinese Academy of Sciences, P.O. Box 1126, Hefei, 230031, P.R. China. lijx@ipp.ac.cn.</nlm:affiliation><country wicri:rule="url">République populaire de Chine</country></affiliation><affiliation wicri:level="1"><nlm:affiliation>Collaborative Innovation Center of Radiation Medicine of Jiangsu Higher Education Institutions, Suzhou, P.R. 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Box 1126, Hefei, 230031, P.R. China.</nlm:affiliation><country xml:lang="fr" wicri:curation="lc">République populaire de Chine</country><wicri:regionArea>Institute of Plasma Physics, Chinese Academy of Sciences, P.O. Box 1126, Hefei, 230031</wicri:regionArea><wicri:noRegion>230031</wicri:noRegion></affiliation><affiliation wicri:level="1"><nlm:affiliation>University of Science and Technology of China, Hefei, 230026, P.R. China.</nlm:affiliation><country xml:lang="fr" wicri:curation="lc">République populaire de Chine</country><wicri:regionArea>University of Science and Technology of China, Hefei, 230026</wicri:regionArea><wicri:noRegion>230026</wicri:noRegion></affiliation></author><author><name sortKey="Sun, Ju" sort="Sun, Ju" uniqKey="Sun J" first="Ju" last="Sun">Ju Sun</name><affiliation wicri:level="1"><nlm:affiliation>Institute of Plasma Physics, Chinese Academy of Sciences, P.O. Box 1126, Hefei, 230031, P.R. China.</nlm:affiliation><country xml:lang="fr" wicri:curation="lc">République populaire de Chine</country><wicri:regionArea>Institute of Plasma Physics, Chinese Academy of Sciences, P.O. Box 1126, Hefei, 230031</wicri:regionArea><wicri:noRegion>230031</wicri:noRegion></affiliation><affiliation wicri:level="1"><nlm:affiliation>University of Science and Technology of China, Hefei, 230026, P.R. China.</nlm:affiliation><country xml:lang="fr" wicri:curation="lc">République populaire de Chine</country><wicri:regionArea>University of Science and Technology of China, Hefei, 230026</wicri:regionArea><wicri:noRegion>230026</wicri:noRegion></affiliation></author><author><name sortKey="Duan, Shengxia" sort="Duan, Shengxia" uniqKey="Duan S" first="Shengxia" last="Duan">Shengxia Duan</name><affiliation wicri:level="1"><nlm:affiliation>Institute of Plasma Physics, Chinese Academy of Sciences, P.O. Box 1126, Hefei, 230031, P.R. China.</nlm:affiliation><country xml:lang="fr" wicri:curation="lc">République populaire de Chine</country><wicri:regionArea>Institute of Plasma Physics, Chinese Academy of Sciences, P.O. Box 1126, Hefei, 230031</wicri:regionArea><wicri:noRegion>230031</wicri:noRegion></affiliation><affiliation wicri:level="1"><nlm:affiliation>University of Science and Technology of China, Hefei, 230026, P.R. China.</nlm:affiliation><country xml:lang="fr" wicri:curation="lc">République populaire de Chine</country><wicri:regionArea>University of Science and Technology of China, Hefei, 230026</wicri:regionArea><wicri:noRegion>230026</wicri:noRegion></affiliation></author><author><name sortKey="Wang, Yanan" sort="Wang, Yanan" uniqKey="Wang Y" first="Yanan" last="Wang">Yanan Wang</name><affiliation wicri:level="1"><nlm:affiliation>Institute of Plasma Physics, Chinese Academy of Sciences, P.O. Box 1126, Hefei, 230031, P.R. China.</nlm:affiliation><country xml:lang="fr" wicri:curation="lc">République populaire de Chine</country><wicri:regionArea>Institute of Plasma Physics, Chinese Academy of Sciences, P.O. Box 1126, Hefei, 230031</wicri:regionArea><wicri:noRegion>230031</wicri:noRegion></affiliation><affiliation wicri:level="1"><nlm:affiliation>University of Science and Technology of China, Hefei, 230026, P.R. China.</nlm:affiliation><country xml:lang="fr" wicri:curation="lc">République populaire de Chine</country><wicri:regionArea>University of Science and Technology of China, Hefei, 230026</wicri:regionArea><wicri:noRegion>230026</wicri:noRegion></affiliation></author><author><name sortKey="Hayat, Tasawar" sort="Hayat, Tasawar" uniqKey="Hayat T" first="Tasawar" last="Hayat">Tasawar Hayat</name><affiliation wicri:level="1"><nlm:affiliation>NAAM Research Group, Faculty of Science, King Abdulaziz University, Jeddah, 21589, Saudi Arabia.</nlm:affiliation><country xml:lang="fr">Arabie saoudite</country><wicri:regionArea>NAAM Research Group, Faculty of Science, King Abdulaziz University, Jeddah, 21589</wicri:regionArea><wicri:noRegion>21589</wicri:noRegion></affiliation></author><author><name sortKey="Alsaedi, Ahmed" sort="Alsaedi, Ahmed" uniqKey="Alsaedi A" first="Ahmed" last="Alsaedi">Ahmed Alsaedi</name><affiliation wicri:level="1"><nlm:affiliation>NAAM Research Group, Faculty of Science, King Abdulaziz University, Jeddah, 21589, Saudi Arabia.</nlm:affiliation><country xml:lang="fr">Arabie saoudite</country><wicri:regionArea>NAAM Research Group, Faculty of Science, King Abdulaziz University, Jeddah, 21589</wicri:regionArea><wicri:noRegion>21589</wicri:noRegion></affiliation><affiliation wicri:level="1"><nlm:affiliation>Department of Mathematics, Quaid-I-Azam University, Islamabad, 44000, Pakistan.</nlm:affiliation><country xml:lang="fr">Pakistan</country><wicri:regionArea>Department of Mathematics, Quaid-I-Azam University, Islamabad, 44000</wicri:regionArea><wicri:noRegion>44000</wicri:noRegion></affiliation></author><author><name sortKey="Wang, Chengming" sort="Wang, Chengming" uniqKey="Wang C" first="Chengming" last="Wang">Chengming Wang</name><affiliation wicri:level="1"><nlm:affiliation>University of Science and Technology of China, Hefei, 230026, P.R. China.</nlm:affiliation><country xml:lang="fr" wicri:curation="lc">République populaire de Chine</country><wicri:regionArea>University of Science and Technology of China, Hefei, 230026</wicri:regionArea><wicri:noRegion>230026</wicri:noRegion></affiliation></author><author><name sortKey="Li, Jiaxing" sort="Li, Jiaxing" uniqKey="Li J" first="Jiaxing" last="Li">Jiaxing Li</name><affiliation wicri:level="1"><nlm:affiliation>Institute of Plasma Physics, Chinese Academy of Sciences, P.O. Box 1126, Hefei, 230031, P.R. China. lijx@ipp.ac.cn.</nlm:affiliation><country wicri:rule="url">République populaire de Chine</country></affiliation><affiliation wicri:level="1"><nlm:affiliation>Collaborative Innovation Center of Radiation Medicine of Jiangsu Higher Education Institutions, Suzhou, P.R. China. lijx@ipp.ac.cn.</nlm:affiliation><country wicri:rule="url">République populaire de Chine</country></affiliation><affiliation wicri:level="1"><nlm:affiliation>NAAM Research Group, Faculty of Science, King Abdulaziz University, Jeddah, 21589, Saudi Arabia. lijx@ipp.ac.cn.</nlm:affiliation><country xml:lang="fr">Arabie saoudite</country><wicri:regionArea>NAAM Research Group, Faculty of Science, King Abdulaziz University, Jeddah, 21589</wicri:regionArea><wicri:noRegion>21589</wicri:noRegion></affiliation></author></analytic><series><title level="j">Scientific reports</title><idno type="eISSN">2045-2322</idno><imprint><date when="2017" type="published">2017</date></imprint></series></biblStruct></sourceDesc></fileDesc><profileDesc><textClass></textClass></profileDesc></teiHeader><front><div type="abstract" xml:lang="en">In this paper, biochar derived from poplar catkins was used as an economical and renewable adsorbent for adsorption organic and inorganic pollutants such as, dyes, organic compounds, and heavy metal ions from wastewater. Mesoporous activated carbonized poplar catkins (ACPCs) were produced from char as a by-product by carbonized poplar catkins (CPCs). With their high surface area, ACPCs exhibited the maximum adsorption capacities of 71.85 and 110.17 mg/g for the removal of inorganic U(VI) and Co(II). Compared other biochars adsorbents, ACPCs can also adsorb organic pollutants with the maximum adsorption capacities of 534, 154, 350, 148 and 384 mg/g for methylene blue (MB), methyl orange (MO), Congo red (CR), chloramphenicol (CAP) and naphthalene. The adsorption of organic pollutants was fitted with pseudo-first order, pseudo-second order, and intra-particle diffusion kinetic models figure out the kinetic parameters and adsorption mechanisms. Langmuir adsorption isotherm was found to be suitable for Co(II) and U(VI) adsorption and thermodynamic studies indicated adsorption processes to be endothermic and spontaneous. The adsorption process includes both outer-sphere surface complexes and hydrogen-bonding interactions. The results showed that biochar derived from poplar catkins was a potential material to remove pollutants in wastewater.</div></front></TEI><pubmed><MedlineCitation Status="PubMed-not-MEDLINE" Owner="NLM"><PMID Version="1">28855653</PMID><DateCompleted><Year>2019</Year><Month>03</Month><Day>21</Day></DateCompleted><DateRevised><Year>2019</Year><Month>03</Month><Day>21</Day></DateRevised><Article PubModel="Electronic"><Journal><ISSN IssnType="Electronic">2045-2322</ISSN><JournalIssue CitedMedium="Internet"><Volume>7</Volume><Issue>1</Issue><PubDate><Year>2017</Year><Month>08</Month><Day>30</Day></PubDate></JournalIssue><Title>Scientific reports</Title><ISOAbbreviation>Sci Rep</ISOAbbreviation></Journal><ArticleTitle>A Valuable Biochar from Poplar Catkins with High Adsorption Capacity for Both Organic Pollutants and Inorganic Heavy Metal Ions.</ArticleTitle><Pagination><MedlinePgn>10033</MedlinePgn></Pagination><ELocationID EIdType="doi" ValidYN="Y">10.1038/s41598-017-09446-0</ELocationID><Abstract><AbstractText>In this paper, biochar derived from poplar catkins was used as an economical and renewable adsorbent for adsorption organic and inorganic pollutants such as, dyes, organic compounds, and heavy metal ions from wastewater. Mesoporous activated carbonized poplar catkins (ACPCs) were produced from char as a by-product by carbonized poplar catkins (CPCs). With their high surface area, ACPCs exhibited the maximum adsorption capacities of 71.85 and 110.17 mg/g for the removal of inorganic U(VI) and Co(II). Compared other biochars adsorbents, ACPCs can also adsorb organic pollutants with the maximum adsorption capacities of 534, 154, 350, 148 and 384 mg/g for methylene blue (MB), methyl orange (MO), Congo red (CR), chloramphenicol (CAP) and naphthalene. The adsorption of organic pollutants was fitted with pseudo-first order, pseudo-second order, and intra-particle diffusion kinetic models figure out the kinetic parameters and adsorption mechanisms. Langmuir adsorption isotherm was found to be suitable for Co(II) and U(VI) adsorption and thermodynamic studies indicated adsorption processes to be endothermic and spontaneous. The adsorption process includes both outer-sphere surface complexes and hydrogen-bonding interactions. The results showed that biochar derived from poplar catkins was a potential material to remove pollutants in wastewater.</AbstractText></Abstract><AuthorList CompleteYN="Y"><Author ValidYN="Y"><LastName>Liu</LastName><ForeName>Xia</ForeName><Initials>X</Initials><AffiliationInfo><Affiliation>Institute of Plasma Physics, Chinese Academy of Sciences, P.O. Box 1126, Hefei, 230031, P.R. China.</Affiliation></AffiliationInfo><AffiliationInfo><Affiliation>University of Science and Technology of China, Hefei, 230026, P.R. China.</Affiliation></AffiliationInfo></Author><Author ValidYN="Y"><LastName>Sun</LastName><ForeName>Ju</ForeName><Initials>J</Initials><AffiliationInfo><Affiliation>Institute of Plasma Physics, Chinese Academy of Sciences, P.O. Box 1126, Hefei, 230031, P.R. China.</Affiliation></AffiliationInfo><AffiliationInfo><Affiliation>University of Science and Technology of China, Hefei, 230026, P.R. China.</Affiliation></AffiliationInfo></Author><Author ValidYN="Y"><LastName>Duan</LastName><ForeName>Shengxia</ForeName><Initials>S</Initials><AffiliationInfo><Affiliation>Institute of Plasma Physics, Chinese Academy of Sciences, P.O. Box 1126, Hefei, 230031, P.R. China.</Affiliation></AffiliationInfo><AffiliationInfo><Affiliation>University of Science and Technology of China, Hefei, 230026, P.R. China.</Affiliation></AffiliationInfo></Author><Author ValidYN="Y"><LastName>Wang</LastName><ForeName>Yanan</ForeName><Initials>Y</Initials><AffiliationInfo><Affiliation>Institute of Plasma Physics, Chinese Academy of Sciences, P.O. Box 1126, Hefei, 230031, P.R. China.</Affiliation></AffiliationInfo><AffiliationInfo><Affiliation>University of Science and Technology of China, Hefei, 230026, P.R. China.</Affiliation></AffiliationInfo></Author><Author ValidYN="Y"><LastName>Hayat</LastName><ForeName>Tasawar</ForeName><Initials>T</Initials><AffiliationInfo><Affiliation>NAAM Research Group, Faculty of Science, King Abdulaziz University, Jeddah, 21589, Saudi Arabia.</Affiliation></AffiliationInfo></Author><Author ValidYN="Y"><LastName>Alsaedi</LastName><ForeName>Ahmed</ForeName><Initials>A</Initials><AffiliationInfo><Affiliation>NAAM Research Group, Faculty of Science, King Abdulaziz University, Jeddah, 21589, Saudi Arabia.</Affiliation></AffiliationInfo><AffiliationInfo><Affiliation>Department of Mathematics, Quaid-I-Azam University, Islamabad, 44000, Pakistan.</Affiliation></AffiliationInfo></Author><Author ValidYN="Y"><LastName>Wang</LastName><ForeName>Chengming</ForeName><Initials>C</Initials><AffiliationInfo><Affiliation>University of Science and Technology of China, Hefei, 230026, P.R. China.</Affiliation></AffiliationInfo></Author><Author ValidYN="Y"><LastName>Li</LastName><ForeName>Jiaxing</ForeName><Initials>J</Initials><AffiliationInfo><Affiliation>Institute of Plasma Physics, Chinese Academy of Sciences, P.O. Box 1126, Hefei, 230031, P.R. China. lijx@ipp.ac.cn.</Affiliation></AffiliationInfo><AffiliationInfo><Affiliation>Collaborative Innovation Center of Radiation Medicine of Jiangsu Higher Education Institutions, Suzhou, P.R. China. lijx@ipp.ac.cn.</Affiliation></AffiliationInfo><AffiliationInfo><Affiliation>NAAM Research Group, Faculty of Science, King Abdulaziz University, Jeddah, 21589, Saudi Arabia. lijx@ipp.ac.cn.</Affiliation></AffiliationInfo></Author></AuthorList><Language>eng</Language><PublicationTypeList><PublicationType UI="D016428">Journal Article</PublicationType><PublicationType UI="D013485">Research Support, Non-U.S. Gov't</PublicationType></PublicationTypeList><ArticleDate DateType="Electronic"><Year>2017</Year><Month>08</Month><Day>30</Day></ArticleDate></Article><MedlineJournalInfo><Country>England</Country><MedlineTA>Sci Rep</MedlineTA><NlmUniqueID>101563288</NlmUniqueID><ISSNLinking>2045-2322</ISSNLinking></MedlineJournalInfo></MedlineCitation><PubmedData><History><PubMedPubDate PubStatus="received"><Year>2017</Year><Month>02</Month><Day>28</Day></PubMedPubDate><PubMedPubDate PubStatus="accepted"><Year>2017</Year><Month>07</Month><Day>27</Day></PubMedPubDate><PubMedPubDate 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Ahmed" sort="Alsaedi, Ahmed" uniqKey="Alsaedi A" first="Ahmed" last="Alsaedi">Ahmed Alsaedi</name><name sortKey="Li, Jiaxing" sort="Li, Jiaxing" uniqKey="Li J" first="Jiaxing" last="Li">Jiaxing Li</name></country><country name="Pakistan"><noRegion><name sortKey="Alsaedi, Ahmed" sort="Alsaedi, Ahmed" uniqKey="Alsaedi A" first="Ahmed" last="Alsaedi">Ahmed Alsaedi</name></noRegion></country></tree></affiliations></record>Pour manipuler ce document sous Unix (Dilib)
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